New PDF release: Modern Aspects of Electrochemistry

By K. Scott (auth.), Ralph E. White, J. O’M. Bockris, B. E. Conway (eds.)

ISBN-10: 1489917241

ISBN-13: 9781489917249

ISBN-10: 1489917268

ISBN-13: 9781489917263

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60), with the material balance gives C - C + AO - A a-rk{lCA 1 + (kfllkLA) (87) This rearranges to give the exit product concentration as CA CAO - 1 1 + a-rkjt 1 +Dal (88) The current balance for this system is . IT= nlFkflCA 1 + (kjtlkLA) +mFkfd (89) In essence, the use of the CSTR models requires the solution of simultaneous equations. For example for a known value of h, kfl is obtained from Eq. (89) and hence XA is obtained from Eq. (88). A major limitation of-the CSTR is that a large residence time is generally needed when a high degree of conversion is required.

ELECTROANALYTICALEXPERIMENT AND REACTION MODELING This section will focus on a range of established electroanalytical methods used in determining reaction mechanisms and associated rate data for electrochemical-based reactions. The role of numerical methods and digital simulation in this task is an important factor, and their use is now widespread, with several computer packages available for ready implementation. 1. Introduction Early work on the modeling of electrochemical reactions was concerned with the field of electroanalytical chemistry.

This is given by a material balance as CCe =Cep + CBp - CBe (102) 40 K. Scott The concentration CCi is therefore given by CCi = CCO + rCee r+ 1 (103) Equations (94)-(96) can now be solved subject to the mode of contral. ,r) (aY2-kc) + (Y a keCSi 2- ke)C [exp(-kc'l'r) - exp(-aY2'l'r)] + Ai CCi exp(-aY2'l'r) C Ai (106) The concentration CD is found from an overall material balance. For the purpose of this model, we will consider that intermediate C is the desired product. If B were desired, then it would be necessary to reconvert C to B by perhaps reoxidation if C is the reduced state.

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Modern Aspects of Electrochemistry by K. Scott (auth.), Ralph E. White, J. O’M. Bockris, B. E. Conway (eds.)

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